Trimming off the affected leaf will not solve the problem if in fact you do have a calcium deficiency which doesn't even look that bad to me; a pic of the whole plant might help. One leaf only tells so much.
Even if you pulverized the limestone to a fine dust it still needs to be broken down by soil microbes before it can be absorbed by the mycorrhizae fungi attached to your plants root system and then converted to usable sugars through photosynthesis. It will take awhile (think weeks or even months) before whatever calcium contained in the crushed rock you added can be absorbed and used by the plant so it will not help for several weeks or possibly even months. Or you could just give soluble liquid nutrient that is immediately usable by the roots directly.
This is the difference between growing organic and growing with nutrients. Adding dry amendments like crushed stone, minerals, and/or kelp meals, etc to the soil needs time to "cook" in during which time the ph typically drops..."hot" soil. It takes about a month for freshly amended soil to normalize ph by itself.
I know that if you need some fast calcium in a pinch you can use hydrated Epsom salt at about 1 tsp per gal of water. It's cheap and easily found in any health store. Bubble it for an hour+ w/ an airstone to mix it which should help a calcium deficiency if that's what you have. Hydrated D-lime could work also but I warn against using crushed rock from your backyard unless you know for sure the mineral content. Dolomite lime and/or garden gypsum are good sources of cal & mag but you need to add it into the soil way before you put the plants.